聚合力，开新局——《园林》学刊同济大学编辑部揭牌仪式暨学刊发展交流会顺利举行

<正>为集中资源优势,打造顶级期刊,助力学科行业发展,《园林》学刊编辑部与同济大学建筑与城市规划学院景观学系于2022年起正式联合办刊。2022年1月4日,《园林》学刊同济大学编辑部揭牌仪式暨学刊发展交流会在同济大学建筑与城市规划学院C1会议室顺利举行。     

Concentration fluctuation caused by reaction-diffusion coupling near catalytic active sites

The coupling of reaction and diffusion between neighboring active sites in the catalyst pore leads to the spatiotemporal fluctuation in component concentration, which is very important to catalyst performance and hence its optimal design. Molecular dynamics simulation with hard-sphere and pseudo-particle modeling has previously revealed the non-stochastic concentration fluctuation of the reactant/product near isolated active site due to such coupling, using a simple model reaction of A → B in 2D pores. The topic is further developed in this work by studying the concentration fluctuation due to such coupling between neighboring active sites in 3D pores. Two 3D pore models containing an isolated active site and two adjacent active sites were constructed, respectively. For the isolated site, the concentration fluctuation intensifies for larger pores, but the product yield decreases, and for a given pore size, the product yield reaches a peak at a certain reactant concentration. For two neighboring sites, their distance (d) is found to have little effect on the reaction, but significant to the diffusion. For the same reaction competing at both sites, larger d leads to more efficient diffusion and better overall performance. However, for sequential reactions at the two sites, higher overall performance presents at a smaller d. The results should be helpful to the catalyst design and reaction control in the relevant processes.     

Surface Modification of Co3O4 Nanosheets to Promote Peroxymonosulfate Activation for Degradation of Atrazine

Catalysis Letters - This study proposed a new facile route to rational creating oxygen-vacancy (Vo)-rich surface of Co3O4 nanosheets by acetic acid leaching. The acid leached Co3O4 nanosheets was...     

The Boundedness and the Global Mittag-Leffler Synchronization of Fractional-Order Inertial Cohen–Grossberg Neural Networks with Time Delays

Neural Processing Letters - The boundedness and the global Mittag-Leffler synchronization (GMLS) of fractional-order inertial Cohen–Grossberg neural networks (CGNNS) with time delays are...     

快速近似计算Shapley值的归因解释方法

Shapley值归因解释方法虽然能更准确量化解释结果, 但过高的计算复杂度严重影响了该方法的实用性. 本文引入KD树重新整理待解释模型的预测数据, 通过在KD树上插入虚节点, 使之满足TreeSHAP算法的使用条件, 在此基础上提出了KDSHAP方法. 该方法解除了TreeSHAP算法仅能解释树结构模型的限制, 将该算法计算Shapley值的高效性放宽到对所有的黑盒模型的解释中, 同时保证了计算准确度. 通过实验对比分析, KDSHAP方法的可靠性, 以及在解释高维输入模型时的适用性.